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991.
M. Gutowski I. Dabkowska J. Rak S. Xu J.M. Nilles D. Radisic K.H. Bowen Jr 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2002,20(3):431-439
The photoelectron spectra (PES) of anions of uracil-glycine and uracil-phenylalanine complexes reveal broad features with
maxima at 1.8 and 2.0 eV. The results of ab initio density functional B3LYP and second order M?ller-Plesset theory calculations indicate that the excess electron occupies a
π* orbital localized on uracil. The excess electron attachment to the complex can induce a barrier-free proton transfer (BFPT)
from the carboxylic group of glycine to the O8 atom of uracil. As a result, the four most stable structures of the anion of
uracil-glycine complex can be characterized as the neutral radical of hydrogenated uracil solvated by the anion of deprotonated
glycine. The similarity between the PES spectra for the uracil complexes with glycine and phenylalanine suggests that the
BFPT is also operative in the case of the latter anionic species. The BFPT to the O8 atom of uracil may be related to the
damage of nucleic acid bases by low energy electrons because the O8 atom is involved in a hydrogen bond with adenine in the
standard Watson-Crick pairing scheme.
Received 6 April 2002 Published online 13 September 2002 相似文献
992.
993.
Ying Zhang Gang Hu Shigang Chen H.A. Cerdeira 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,27(3):381-384
A method of controlling global stochasticity in Hamiltonian systems by applying nonlinear perturbation is proposed. With the
well-known standard map we demonstrate that this control method can convert global stochasticity into regular motion in a
wide chaotic region for arbitrary initial condition, in which the control signal remains very weak after a few kicks. The
system in which chaos has been controlled approximates to the original Hamiltonian system, and this approach appears robust
against small external noise. The mechanism underlying this high control efficiency is intuitively explained.
Received 15 January 2002 Published online 6 June 2002 相似文献
994.
D.A. Garanin E.M. Chudnovsky 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,28(1):3-7
We compute the width and shape of the EPR and tunneling resonances due to dislocations in Mn12 acetate crystals. Uncorrelated dislocations produce the Gaussian shape of resonances while dislocations bound in pairs produce
the Lorentzian shape. We stress that the uniaxial spin Hamiltonian together with crystal defects can explain the totality
of experimental data on Mn12.
Received 2 August 2001 / Received in final form 15 March 2002 Published online 17 September 2002 相似文献
995.
R. Adhikari A. Sil A. Raychaudhuri 《The European Physical Journal C - Particles and Fields》2002,25(1):125-130
We present a solution of the solar neutrino deficit using three flavors of neutrinos and R-parity non-conserving supersymmetry. In this model, in vacuum, the is massless and unmixed, mass and mixing being restricted to the - sector only, which we choose in consistency with the requirements of the atmospheric neutrino anomaly. The flavor changing
and flavor diagonal neutral currents present in the model and the three-flavor picture together produce an energy dependent
resonance-induced - mixing in the sun. This mixing plays a key role in the new solution to the solar neutrino problem. The best fit to the solar
neutrino rates and spectrum (1258-day SK and 241-day SNO data) requires a mass square difference of eV2 in vacuum between the two lightest neutrinos. This solution cannot accommodate a significant day-night effect for solar neutrinos
nor CP violation in terrestrial neutrino experiments.
Received: 26 December 2001 / Revised version: 16 February 2002 / Published online: 26 July 2002 相似文献
996.
The object of the present investigation is to introduce a new trigonometric method of summation which is both regular and
Fourier effective and determine its status with reference to other methods of summation (see §2-§4) and also give an application
of this method to determine the degree of approximation in a new Banach space of functions conceived as a generalized Holder
metric (see §5). 相似文献
997.
It was found that a beta-fructofuranosidase produced by Microbacterium sp. H-1 has potent trans-beta-fructofuranosylation activity from sucrose (donor). By means of this enzyme system, rebaudioside A (RA), the second major sweet steviol glycoside of the leaves of Stevia rebaudiana, was subjected to transfructosylation, affording a mono-beta-fructofuranosylated product (RA-F) in a high yield. The structure of RA-F was elucidated as beta-D-fructofuranosyl-(2----6)-beta-D-glucopyranosyl ester of steviol-13-O-[beta-D-glucopyranosyl-(1----2)]- [beta-D-glucopyranosyl-(1----3)]-beta-D-glucopyranoside. Some improvement in the quality of sweetness was observed for RA-F. 相似文献
998.
By an elementary calculation we obtain the exact mean values of Minkowksi functionals for a standard model of percolating sets. In particular, a recurrence theorem for the mean Euler characteristic recently put forward is shown to be incorrect. Related previous mathematical work is mentioned. We also conjecture bounds for the threshold density of continuum percolation, which are associated with the Euler characteristic. 相似文献
999.
B. A. Usievich D. Kh. Nurligareev V. A. Sychugov K. M. Golant 《Optics and Spectroscopy》2006,101(6):930-934
A system of tunnel-coupled rectilinear waveguides is studied. The dependence of the number of modes in this system on the number of waveguides N, the distance between the waveguides, and the number of modes in a separate waveguide is considered. It is shown that the modes of the m = N and N + 1 orders in such a system are Bragg modes; i.e., the angle between the direction of their propagation and the system axis is close to the Bragg angle. The effective refractive indices n * of these modes change stepwise. The step size Δn * is found to be dependent on the distance s between the waveguides and on the number of modes in a separate waveguide. A system of single-mode waveguides with the number of guided modes M = 34 < N = 50 is studied experimentally. It is shown that the Bragg modes of the system lie among the leakage modes of the system and have rather low losses. It is demonstrated that the localization of the Bragg modes among the leakage modes may be favorable for their selection upon light generation. 相似文献
1000.
Water suppression by diffusive attenuation was used to measure Brix in intact cellular tissue of apple and strawberry. Given
the signal-to-noise ratio, the correlation for apple was established without repeated acquisition, so this protocol should
also be useful for rapid, on-line measurements at low spectrometer frequencies. Water suppression by theT
1-Null method fails with cellular tissue because of the considerable variation in the longitudinal relaxation times of vacuolar
and cytoplasmic water. 相似文献